Chiral superconductivity in UTe probed by anisotropic low-energy excitations

Ishihara, Kota*; Roppongi, Masaki*; Kobayashi, Masayuki*; Imamura, Kumpei*; Mizukami, Yuta*; Sakai, Hironori; Opletal, P.; Tokiwa, Yoshifumi; Haga, Yoshinori; Hashimoto, Kenichiro*; et al.

Nature Communications (Internet), 14, p.2966_1 - 2966_7, 2023/05

https://doi.org/10.1038/s41467-023-38688-y

The superconducting symmetry of the heavy fermion uranium-based superconductor UTe is investigated using low temperature penetration depth measurements. The anisotropic low-energy quasiparticle excitations indicates multiple superconducting components in a chiral complex form. The most consistent is a chiral non-unitary state.

Chapter 5, Sodium-cooled Fast Reactor (SFRs)/ Chapter 12, Generation-IV Sodium-cooled Fast Reactor (SFR) concepts in Japan

Kubo, Shigenobu; Chikazawa, Yoshitaka; Ohshima, Hiroyuki; Kamide, Hideki

Handbook of Generation IV Nuclear Reactors, Second Edition, p.173 - 194, 2023/03

Handbook of Generation IV Nuclear Reactors, Second Edition is a fully revised and updated comprehensive resource on the latest research and advances in generation IV nuclear reactor concepts. Editor Igor Pioro and his team of expert contributors have updated every chapter to reflect advances in the field since the first edition published in 2016. JAEA contributes to Chapter 5; Sodium-cooled Fast Reactors (SFRs) and Chapter 12; Generation-IV Sodium-cooled Fast Reactor (SFR) concepts in Japan. Major characteristics and current technology developments including safety enhancement were described in Chapter 5. Chapter 12 shows design activities of SFR. Innovative technology developments, and update of the Japan sodium-cooled fast reactor design with lessons learned from the TEPCO Fukushima Daiichi NPP accident.

Decrease of radionuclide sorption in hydrated cement systems by organic ligands; Comparative evaluation using experimental data and thermodynamic calculations for ISA/EDTA-actinide-cement systems

Ochs, M.*; Dolder, F.*; Tachi, Yukio

Applied Geochemistry, 136, p.105161_1 - 105161_11, 2022/01

https://doi.org/10.1016/j.apgeochem.2021.105161

Various types of radioactive wastes and environments contain organic substances that can stabilize the aqueous complexes with radionuclides and therefore lead to a decrease of sorption. The present study focuses on testing a methodology to quantify sorption reduction factors (SRFs) in the presence of organic ligands for cement systems. Three approaches for the estimation of SRFs; (1) analogy with solubility enhancement factors, (2) radionuclide speciation based on the thermodynamic calculations, and (3) experimental sorption data in ternary systems, were coupled and tested for the representative organic ligands (ISA and EDTA) and selected key radionuclides (actinides). Our approach allows to critically evaluate the dependence of SRFs for various systems on the chosen method of quantification, in accordance with the data availability for a given systems. The reliable SRFs can only be derived from the sorption measurements in ternary systems. SRF often need to be derived in the absence of such direct evidence, and estimations need to be made based on analogies and speciation information. However, such estimates may be subject to substantial uncertainties.

Momentum dependence of Mott gap excitations in optimally doped YBaCuO studied by resonant inelastic X-ray scattering

Ishii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Kuzushita, Kaori; Inami, Toshiya; Owada, Kenji; Maekawa, Sadamichi*; Masui, Takahiko*; Tajima, Setsuko*; et al.

AIP Conference Proceedings 850, p.445 - 446, 2006/09

https://doi.org/10.1063/1.2354776

Mott gap excitations in the optimally doped high- superconductor YBaCuO ( = 93 K) have been studied by the resonant inelastic X-ray scattering method. Anisotropic spectra in the -plane are observed in a twin-free crystal. The excitation from the one-dimensional CuO chain is enhanced at 2 eV near the zone boundary of the direction, while the excitation from the CuO plane is broad at 1.5-4 eV and almost independent of the momentum transfer. Theoretical calculation based on the one-dimensional and two-dimensional Hubbard model reproduces the observed spectra when different values of the on-site Coulomb energy are assumed. The Mott gap of the CuO chain site is found to be much smaller than that of the CuO plane site.

Electronic excitations in hole-doped LaSrMnO studied by resonant inelastic X-ray scattering

Ishii, Kenji; Inami, Toshiya; Owada, Kenji; Kuzushita, Kaori; Mizuki, Junichiro; Murakami, Yoichi; Ishihara, Sumio*; Endo, Yasuo*; Maekawa, Sadamichi*; Hirota, Kazuma*; et al.

Journal of Physics and Chemistry of Solids, 66(12), p.2157 - 2162, 2005/12

https://doi.org/10.1016/j.jpcs.2005.09.011

We have studied electronic excitations of hole-doped manganese oxides LaSrMnO ( and ) by resonant inelastic X-ray scattering at Mn K absorption edge. We observed in the excitation spectra that the Mott gap of LaSrMnO was filled by hole-doping. In LaSrMnO, which shows a metal-insulator transition, we found that temperature dependence of scattering intensity is different between two scattering vectors. It may reflects a anisotropic electronic structure which originates from the orbital degrees of freedom in manganese oxides.

Momentum dependence of charge excitations in the electron-doped superconductor NdCeCuO; A Resonant inelastic X-ray scattering study

Ishii, Kenji; Tsutsui, Kenji*; Endo, Yasuo*; Toyama, Takami*; Maekawa, Sadamichi*; Hoesch, M.; Kuzushita, Kaori; Tsubota, Masami; Inami, Toshiya; Mizuki, Junichiro; et al.

Physical Review Letters, 94(20), p.207003_1 - 207003_4, 2005/05

https://doi.org/10.1103/PhysRevLett.94.207003

We report a resonant inelastic X-ray scattering (RIXS) study of charge excitations in the electron-doped high- superconductor NdCeCuO. The intraband and interband excitations across the Fermi energy are separated for the first time by tuning the experimental conditions properly to measure charge excitations at low energy. A dispersion relation with -dependent width emerges clearly in the intraband excitation, while the intensity of the interband excitation is concentrated around 2 eV near the zone center. The experimental results are consistent with theoretical calculation of the RIXS spectra based on the Hubbard model.

Resonant inelastic X-ray scattering study of the hole-doped manganites LaSrMnO (, )

Ishii, Kenji; Inami, Toshiya; Owada, Kenji; Kuzushita, Kaori; Mizuki, Junichiro; Murakami, Yoichi; Ishihara, Sumio*; Endo, Yasuo*; Maekawa, Sadamichi*; Hirota, Kazuma*; et al.

Physical Review B, 70(22), p.224437_1 - 224437_6, 2004/12

https://doi.org/10.1103/PhysRevB.70.224437

Electronic excitations in the hole doped manganese oxides (LaSrMnO, and ) have been elucidated by using the resonant inelastic X-ray scattering (RIXS) method. A doping effect in the strongly correlated electron systems has been observed for the first time. The scattering spectra show that a salient peak appears in low energies indicating the persistence of the Mott gap. At the same time, the energy gap is partly filled by doping holes and the spectral weight energy shifts toward lower energies. The excitation spectra show little change in the momentum space as is in undoped LaMnO. On the other hand, the scattering intensities in the low energy excitations of are anisotropic in temperature dependence, which indicates an anisotropy of magnetic interaction and underlying effect of the orbital.

Theory of superconductivity in strongly correlated electron systems

Yanase, Yoichi*; Jujo, Takanobu*; Nomura, Takuji; Ikeda, Hiroaki*; Hotta, Takashi; Yamada, Kosaku*

Physics Reports; A Review Section of Physics Letters, 387(1-4), p.1 - 149, 2003/11

https://doi.org/10.1016/j.physrep.2003.07.002

In this article we review essential natures of superconductivity in strongly correlated electron systems from a universal point of view. Here we consider materials such as high- cuprates, BEDT-TTF organic superconductors, ruthenate SrRuO, and heavy fermion superconductors. After the review of experimental results, we explain the formalism to discuss superconducting properties of strongly correlated electron systems based on the Dyson-Gor'kov equations. Then, we introduce theoretical retults on cuprates, organics, ruthenate, and heavy fermion superconductors in this order.

Data analysis on worker dose in dismantling of Japan Power Demonstration Reactor (JPDR) (Contract research)

Shiraishi, Kunio; Sukegawa, Takenori; Yanagihara, Satoshi

JAERI-Data/Code 2001-028, 86 Pages, 2001/11

JAERI-Data-Code-2001-028.pdf:6.31MB

The data on worker dose in dismantling of the Japan Power Demonstration Reactor (JPDR) was analyzed to characterize its features. It was appeared from the study that the collective dose to the workers was 306 man-mSv, in which maximum individual dose was 8.5 mSv, almost all doses were received in the activities for dismantling of reactor internals, the reactor pressure vessel and the biological shield, and that the worker dose distribution was similar to that in the maintenanee of the facilities which was characterized by the hybrid log normal distribution model. Farthermore, it was found that the dismantling activities were categorized into three groups depending on dose rates in workplaces, then contribution factors for radiation exposure in terms of dose rates in different groups were derived based on the analysis. The study would be useful for estimation of worker dose in future decommissioning of commercial nuclear power plants in Japan.

Data analysis on waste arising in dismantling of Japan Power Demonstration Reactor (JPDR) (Contract research)

Shiraishi, Kunio; Sukegawa, Takenori; Yanagihara, Satoshi

JAERI-Data/Code 99-050, p.113 - 0, 2000/01

JAERI-Data-Code-99-050.pdf:5.95MB

no abstracts in English